There are many NGO's where you can make a call and they themselves come and pick up the things or you can yourself too drop them. If you find it little cumbersome, the best way, that I generally do is, donate things to our society guards or maids. There is so much of labour around, you can politely ask if they have little ones and home and you would like to giveaway a few things. And if you think you might be offending someone, you can put it other way as, "There are little baby's items that I want to give away, you see many help crossing, if you come across who is in need, you can send her to my place to collect it." http://greenyatra.org/zaroorat/ http://www.adarshmay.org There are plenty of other NGO's too that you can find if you go through the Internet, which may be close by the area you live in.
Hey thats a great gesture you are thinking of. If you are looking at donating toys that are in good condition, you can check out an organization called Toybank that helps reach out toys to children in need. Also, you can donate clothes and other items to local orphanages, that often take in such things.
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